Hyperfine characterization of tin-doped indium sesquioxide
Identifieur interne : 000684 ( Main/Exploration ); précédent : 000683; suivant : 000685Hyperfine characterization of tin-doped indium sesquioxide
Auteurs : RBID : ISTEX:10751_1985_Article_BF02058077.pdfAbstract
The hyperfine interactions at In and Sn sites of In2O3∶Sn (ITO) were measured through time-differential perturbed angular correlations and Mössbauer spectroscopy, respectively. Polycrystalline samples prepared by co-precipitation with nominal 0.025, 1 and 5 at.% Sn were studied. They all showed the cubic bixbyite structure characteristic of In2O3 after annealings at 200 °C. The quadrupole interaction at In sites appears nearly independent of Sn concentration being the main result of the presence of Sn in the lattice, the gradual disappearence of the dynamic perturbation caused by after-effects. The Mössbauer data demonstrate that Sn ions are in a 4+ state with ΔQ=0.606 mm/s andδ=0.226 mm/s relative to SnO3Ca at room temperature.
DOI: 10.1007/BF02058077
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Sánchez</name><affiliation wicri:level="1"><mods:affiliation>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata, Argentina</mods:affiliation><country xml:lang="fr">Argentine</country><wicri:regionArea>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata</wicri:regionArea><wicri:noRegion>La Plata</wicri:noRegion></affiliation></author><author><name>L. A. Mendoza-Zélis</name><affiliation wicri:level="1"><mods:affiliation>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata, Argentina</mods:affiliation><country xml:lang="fr">Argentine</country><wicri:regionArea>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata</wicri:regionArea><wicri:noRegion>La Plata</wicri:noRegion></affiliation></author><author><name>L. Terminiello</name><affiliation wicri:level="1"><mods:affiliation>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata, Argentina</mods:affiliation><country xml:lang="fr">Argentine</country><wicri:regionArea>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata</wicri:regionArea><wicri:noRegion>La Plata</wicri:noRegion></affiliation></author><author><name>A. G. Bibiloni</name><affiliation wicri:level="1"><mods:affiliation>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata, Argentina</mods:affiliation><country xml:lang="fr">Argentine</country><wicri:regionArea>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata</wicri:regionArea><wicri:noRegion>La Plata</wicri:noRegion></affiliation></author><author><name>C. P. Massolo</name><affiliation wicri:level="1"><mods:affiliation>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata, Argentina</mods:affiliation><country xml:lang="fr">Argentine</country><wicri:regionArea>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata</wicri:regionArea><wicri:noRegion>La Plata</wicri:noRegion></affiliation></author><author><name>J. Desimoni</name><affiliation wicri:level="1"><mods:affiliation>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata, Argentina</mods:affiliation><country xml:lang="fr">Argentine</country><wicri:regionArea>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata</wicri:regionArea><wicri:noRegion>La Plata</wicri:noRegion></affiliation></author><author><name>A. R. López-García</name><affiliation wicri:level="1"><mods:affiliation>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata, Argentina</mods:affiliation><country xml:lang="fr">Argentine</country><wicri:regionArea>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata</wicri:regionArea><wicri:noRegion>La Plata</wicri:noRegion></affiliation></author></titleStmt><publicationStmt><idno type="RBID">ISTEX:10751_1985_Article_BF02058077.pdf</idno><date when="1985">1985</date><idno type="doi">10.1007/BF02058077</idno><idno type="wicri:Area/Main/Corpus">000769</idno><idno type="wicri:Area/Main/Curation">000769</idno><idno type="wicri:Area/Main/Exploration">000684</idno></publicationStmt></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="eng">The hyperfine interactions at In and Sn sites of In2O3∶Sn (ITO) were measured through time-differential perturbed angular correlations and Mössbauer spectroscopy, respectively. Polycrystalline samples prepared by co-precipitation with nominal 0.025, 1 and 5 at.% Sn were studied. They all showed the cubic bixbyite structure characteristic of In2O3 after annealings at 200 °C. The quadrupole interaction at In sites appears nearly independent of Sn concentration being the main result of the presence of Sn in the lattice, the gradual disappearence of the dynamic perturbation caused by after-effects. The Mössbauer data demonstrate that Sn ions are in a 4+ state with ΔQ=0.606 mm/s andδ=0.226 mm/s relative to SnO3Ca at room temperature.</div></front></TEI><mods xsi:schemaLocation="http://www.loc.gov/mods/v3 file:///applis/istex/home/loadistex/home/etc/xsd/mods.xsd" version="3.4" istexId="84adcea9a9aead0642f1b159d96dd5d272893786"><titleInfo lang="eng"><title>Hyperfine characterization of tin-doped indium sesquioxide</title></titleInfo><name type="personal"><namePart type="given">R. C.</namePart><namePart type="family">Mercader</namePart><role><roleTerm type="text">author</roleTerm></role><affiliation>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata, Argentina</affiliation></name><name type="personal"><namePart type="given">F. H.</namePart><namePart type="family">Sánchez</namePart><role><roleTerm type="text">author</roleTerm></role><affiliation>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata, Argentina</affiliation></name><name type="personal"><namePart type="given">L. A.</namePart><namePart type="family">Mendoza-Zélis</namePart><role><roleTerm type="text">author</roleTerm></role><affiliation>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata, Argentina</affiliation></name><name type="personal"><namePart type="given">L.</namePart><namePart type="family">Terminiello</namePart><role><roleTerm type="text">author</roleTerm></role><affiliation>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata, Argentina</affiliation></name><name type="personal"><namePart type="given">A. G.</namePart><namePart type="family">Bibiloni</namePart><role><roleTerm type="text">author</roleTerm></role><affiliation>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata, Argentina</affiliation></name><name type="personal"><namePart type="given">C. 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R.</namePart><namePart type="family">López-García</namePart><role><roleTerm type="text">author</roleTerm></role><affiliation>Departmento de Física, Facultad de Ciencias Exactas, Universidad Universidad Nacional de La Plata, Calle 49 y 115, 1900, La Plata, Argentina</affiliation></name><typeOfResource>text</typeOfResource><genre>Original Paper</genre><originInfo><publisher>Kluwer Academic Publishers, Dordrecht</publisher><dateCreated encoding="w3cdtf">1985-01-10</dateCreated><dateValid encoding="w3cdtf">2005-07-24</dateValid><copyrightDate encoding="w3cdtf">1985</copyrightDate></originInfo><language><languageTerm type="code" authority="iso639-2b">eng</languageTerm></language><physicalDescription><internetMediaType>text/html</internetMediaType></physicalDescription><abstract lang="eng">The hyperfine interactions at In and Sn sites of In2O3∶Sn (ITO) were measured through time-differential perturbed angular correlations and Mössbauer spectroscopy, respectively. Polycrystalline samples prepared by co-precipitation with nominal 0.025, 1 and 5 at.% Sn were studied. They all showed the cubic bixbyite structure characteristic of In2O3 after annealings at 200 °C. The quadrupole interaction at In sites appears nearly independent of Sn concentration being the main result of the presence of Sn in the lattice, the gradual disappearence of the dynamic perturbation caused by after-effects. The Mössbauer data demonstrate that Sn ions are in a 4+ state with ΔQ=0.606 mm/s andδ=0.226 mm/s relative to SnO3Ca at room temperature.</abstract><relatedItem type="series"><titleInfo type="abbreviated"><title>Hyperfine Interact</title></titleInfo><titleInfo><title>Hyperfine Interactions</title><partNumber>Year: 1985</partNumber><partNumber>Volume: 23</partNumber><partNumber>Number: 2</partNumber></titleInfo><genre>Archive Journal</genre><originInfo><dateIssued encoding="w3cdtf">1985-09-01</dateIssued><copyrightDate encoding="w3cdtf">1985</copyrightDate></originInfo><subject usage="primary"><topic>Physics</topic><topic>Nuclear Physics, Heavy Ions, Hadrons</topic><topic>Atoms, Molecules, Clusters and Plasmas</topic><topic>Condensed Matter</topic><topic>Surfaces and Interfaces, Thin Films</topic></subject><identifier type="issn">0304-3843</identifier><identifier type="issn">Electronic: 1572-9540</identifier><identifier type="matrixNumber">10751</identifier><identifier type="local">IssueArticleCount: 7</identifier><recordInfo><recordOrigin>J.C. Baltzer AG, Scientific Publishing Company, 1985</recordOrigin></recordInfo></relatedItem><identifier type="doi">10.1007/BF02058077</identifier><identifier type="matrixNumber">Art5</identifier><identifier type="local">BF02058077</identifier><accessCondition type="use and reproduction">MetadataGrant: OpenAccess</accessCondition><accessCondition type="use and reproduction">AbstractGrant: OpenAccess</accessCondition><accessCondition type="restriction on access">BodyPDFGrant: Restricted</accessCondition><accessCondition type="restriction on access">BodyHTMLGrant: Restricted</accessCondition><accessCondition type="restriction on access">BibliographyGrant: Restricted</accessCondition><accessCondition type="restriction on access">ESMGrant: Restricted</accessCondition><part><extent unit="pages"><start>211</start><end>220</end></extent></part><recordInfo><recordOrigin>J.C. Baltzer A.G., Scientific Publishing Company, 1985</recordOrigin><recordIdentifier>10751_1985_Article_BF02058077.pdf</recordIdentifier></recordInfo></mods></record>Pour manipuler ce document sous Unix (Dilib)
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